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HPSynR Research Interests


The group develops high-pressure science as a powerful and clean tuning dimension to explore emergent phenomena in quantum and functional materials, discover metastable states, and probe matter under extreme conditions.

1. Quantum Materials under Pressure

高压调控量子材料:超导、电荷序与拓扑相变

The group investigates the evolution of quantum states under pressure, leveraging pressure as a continuous and chemical-free tuning parameter to uncover the interplay between superconductivity, topological transitions, charge ordering, and magnetism in correlated materials. Significant advances have been achieved in nickelates, layered transition metal chalcogenides, and quasi-one-dimensional systems, highlighting the group's strength in discovering and understanding emergent quantum states under pressure.

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2. Pressure-Engineered Functional Materials

压力工程功能材料:光电、发光、非线性光学与铁电光伏

The group extends high-pressure techniques to functional materials, systematically tuning band structures, local coordination environments, excitonic behaviors, symmetry breaking, and ferroelectric relaxation dynamics. This has led to the development of a “pressure engineering” strategy for enhancing material functionalities, including improved luminescence, optoelectronic response, nonlinear optical properties, and ferroelectric photovoltaic effects in halide perovskites and related systems.

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3. Metastable Materials and High-Pressure Synthesis

高压诱导新材料与亚稳相合成:从新结构发现到常压保留

A central focus of the group is the discovery of new structures and phases under pressure, along with understanding their kinetic pathways and stabilization mechanisms. The group aims to translate high-pressure phases into recoverable metastable materials at ambient conditions, enabling practical applications. Notable achievements include the synthesis of bulk hexagonal diamond, metastable polymorphs, and strategies for retaining high-pressure phases.

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4. Dynamic Compression and Extreme States of Matter

动态压缩与极端条件原位表征:面向地学与超高压前沿

Beyond static compression, the group explores materials under shock compression and laser-driven extreme conditions, employing time-resolved techniques to probe structural evolution on nanosecond timescales. These studies contribute to understanding materials behavior relevant to geophysics, planetary science, and warm dense matter, bridging condensed matter physics and extreme environment science.

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5. High-Pressure Methods and In Situ Characterization

高压实验方法与多场耦合原位表征平台

The group actively develops multi-field coupled experimental platforms integrating high pressure, low temperature, and time-resolved in situ probes. These methodological advances enable precise calibration, structural determination, and dynamic measurements, providing critical tools for studying complex materials under extreme conditions.

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Research - High Pressure Physics Group

Research Directions

HP-LT Transport AC Susceptibility HP-XRD DAC

1. High-pressure Superconductivity in Nickelates and Hydrides

Superconductivity in pressurized trilayer La₄Ni₃O₁₀ single crystals PDF

Nature 631, 531 (2024)

Discovery: Bulk superconductivity in pressurized trilayer La₄Ni₃O₁₀ single crystals.

Solution: Whether nickelates exhibit bulk high-Tc superconductivity similar to cuprates.

Bulk superconductivity in pressurized Pr₄Ni₃O₁₀ PDF Media

Phys. Rev. X 15, 021008 (2025)

Discovery: Bulk superconductivity in Pr₄Ni₃O₁₀ under high pressure.

Solution: Universality of superconductivity across rare-earth elements in trilayer nickelates.

Superconductivity in La₄Ni₃O₁₀ under pressure PDF

Phys. Rev. X 15, 021005 (2025)

Discovery: Consistent superconducting signatures across independent measurements.

Solution: Sample quality and experimental artifact concerns through cross-validation.

Identification of superconductivity in bilayer La₃Ni₂O₇ upon 100 GPa PDF

National Science Review (2025)

Discovery: High-Tc superconductivity in bilayer La₃Ni₂O₇ up to 100 GPa.

Solution: Pressure range and phase diagram for the bilayer nickelate system.

[Image of Atomic Structure]
Synchrotron XRD PDF HR-TEM APT

2. Atomic Structure of Metallic Glasses

Long-Range Topological Order in Metallic Glass PDF Media

Science 332, 1404 (2011)

Discovery: Long-range topological order in metallic glasses.

Solution: Long-standing puzzle of medium-range order hidden in metallic glasses.

Universal Fractional Power Law for Density PDF

Phys. Rev. Lett. 112, 185502 (2014)

Discovery: Universal 2.5 power law governing density scaling under compression.

Solution: Lack of unified description for compression behavior of diverse MG systems.

HP-XPCS Ultrasonic Fast DSC

3. Structure/Properties Tuning under High Pressure

Sub-direction: Relaxation & Free Volume

Nonmonotonic crossover of relaxation dynamics PDF

PNAS 120, e2302281120 (2023)

Discovery: Nonmonotonic crossover of atomic relaxation dynamics under high pressure.

Permanent annihilation of free volume in La₇₅Al₂₅

Phys. Rev. B 109, 214201 (2024)

Solution: Post-processing control over structural relaxation and mechanical properties.

Sub-direction: Two-way Tuning

Two-way tuning of structural order in metallic glasses PDF

Nat. Commun. 11, 314 (2020)

Solution: Reversible "order ↔ disorder" control in amorphous materials.

LVP Laser-Heated DAC SEM/EELS

8. Novel Materials Synthesis

Preservation of high-pressure volatiles in diamond capsules PDF Media

Nature 608, 513 (2022)

Discovery: "Nanostructured diamond capsules" that permanently preserve HP states at ambient conditions.

Solution: Century-long problem that HP phases only exist inside pressure apparatus.

Synthesis of glassy diamond PDF

Nat. Commun. 8, 322 (2017)

Discovery: Completely new carbon material – glassy diamond.

HP-XPCS Transport Setup Synchrotron Laue

9. Development of Novel Techniques

Sub-direction: In-situ HP Wide-Angle XPCS

In situ HP wide-angle hard XPCS: A versatile tool

Matter Radiat. Extremes 8, 028101 (2023)

Solution: Directly observing atomic-scale relaxation dynamics under extreme conditions.

Sub-direction: HP-LT Transport Diagnostic

Origin of resistance transition in Lu-H-N

National Science Review (2023)

Discovery: Resistance jump in Lu-H-N is NOT superconductivity but metal-to-poor-conductor transition.

Solution: Definitive diagnostic method to distinguish true superconductivity from false positives.

Lab Capabilities & Infrastructure

Advanced Experimental Platforms

NMR Spectroscopy

Capabilities

  • • Solid-state NMR
  • • High-pressure In-situ Cell

Key Parameters

Frequency: 600 MHz

Temp: 1.5K - 400K

Low-Temperature Raman

Optical spectroscopy system for vibrational analysis under cryo-conditions.

In-situ HP Mapping Variable Laser Lines

Extreme HP Platforms

Pressure Range Up to 300 GPa+
Heating Method In-situ Laser Heating

Comprehensive expertise in Diamond Anvil Cell (DAC) technology and Synchrotron coupling.

Synchrotron Integration

Stable collaboration with global facilities for XRD, XAFS, and XPCS atomic dynamic probing.